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Vehicle-Based Methane Detection, Attribution, and Quantification in the Upstream Oil and Gas Sector: Method Overview and Controlled Release Validation
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Abstract
Vehicle-based measurement systems occupy an important niche in the multi-scale methane measurement landscape between component-level technologies (e.g. OGI) and aerial-based methods. Performance evaluations are often limited to one dimension (e.g. quantification), while methodological opacity limits interpretation and inter-comparisons between technologies. Here, we develop a vehicle-based measurement system and processing framework incorporating a novel weighted likelihood algorithm for automated source attribution. Using controlled release experiments at two dedicated testing facilities, we characterize system performance across three dimensions – detection, attribution, and quantification. The system achieved a 96.1 % true positive detection rate with no false positives and a 90% detection limit as low as 0.024 kg/h with repeat transects. Attribution accuracy was high at the source-group level, reaching 99.7 % in single-source releases and 86 % in multi-source scenarios. Quantification was unbiased for low-to-moderate complexity releases (2 source groups; slope=0.99, R2=0.81) but overestimated under highly complex conditions (5 source groups; slope=1.45, R2=0.91). These results provide a transparent performance benchmark, demonstrating that these systems are well-suited to survey the large populations of low-to-moderate complexity sites (e.g. single wells and batteries), as a screening layer in LDAR applications and to quantify the low-end of emission distributions in inventories, reducing reliance on generic emission factors.
DOI
https://doi.org/10.31223/X5WZ04
Subjects
Environmental Sciences
Keywords
methane detection, vehicle-based measurement, emission quantification, controlled release experiment, source attribution
Dates
Published: 2026-05-04 09:30
Last Updated: 2026-05-04 09:30
License
CC-BY Attribution-NonCommercial 4.0 International
Additional Metadata
Conflict of interest statement:
None
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